Chinese Journal of Quantum Electronics ›› 2024, Vol. 41 ›› Issue (6): 970-980.doi: 10.3969/j.issn.1007-5461.2024.06.013

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Spontaneous radiation properties of graphene⁃based core⁃shell structure

SHI Shenxi 1 , WANG Zuohong 1 , SUN Mengran 1 , ZHENG Gaige 1,2*   

  1. 1 School of Physics and Optoelectronic Engineering, Nanjing University of Information Science & Technology, Nanjing 210044, China; 2 Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment Technology, Nanjing University of Information Science & Technology, Nanjing 210044, China
  • Received:2022-11-16 Revised:2022-11-30 Published:2024-11-28 Online:2024-11-28

Abstract: To study the scattering properties of core-shell structure containing graphene, expecially electric field distribution, energy density, and radiative/nonradiative decay rate properties, the transfer matrix method (TMM) is used to evaluate the effects of wavelength of the incident ray and dipole emitter location on the spontaneous radiation of Au@SiO2@Graphene. It is found that when the core size and shell thickness remain constant, the Purcell factor in the near-field region of the core-shell structure increases with the increase of the thickness of the intermediate SiO2 dielectric layer. And the Purcell factor of the core-shell structure decreases with the distance of the dipole emitter from the center of the sphere, realizing the regulation of spontaneous radiation. On the other hand, by optimizing the structural parameters of graphene-based core-shell structure, the maximum value of the Purcell factor in the visible light range is achieved at about 633 nm. When the thickness of the dielectric layer is fixed, increasing the radius of the model will lead to a decrease of the Purcell factor. And changing the size parameters of the model can effectively strengthen the interaction between the graphene-based core-shell structure with light wave. The research can provide a reference for the solar thermal field.

Key words: 光电子学, 自发辐射, 传输矩阵, 核壳结构, 石墨烯

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